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One three-dimensional Gd(III) coordination polymer with 1,2-phenylenediacetate exhibiting ferromagnetic interaction and large magnetocaloric effect

One three-dimensional Gd(III) coordination polymer with 1,2-phenylenediacetate (PDA2?), [Gd2(PDA)3(H2O)2]·3H2O (1), has been successfully synthesized and characterized. Single crystal X-ray diffraction analysis shows that 1 consists of 1D wave Gd-based chain unit and PDA2? linker. Magnetic studies suggest the presence of ferromagnetic Gd?Gd coupling in the 1D chain unit of 1. Meanwhile, 1 has a significant cryogenic magnetocaloric effect with the maximum ??Sm of 33.44 at 2K and 7T.

» Author: Zhong-Yi Li, Jing-Yu Li, Lian-Lian Pei, Xiang-Fei Zhang, Guang-Xiu Cao, Chi Zhang, Su-Zhi Li, Bin Zhai

» Reference: Inorganic Chemistry Communications, Volume 87

» Publication Date: 01/01/2018

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